I think that most automotive engines used cast iron crankshafts on their standard performance models. Some times the crank pins and journals were induction hardened on them. The cast iron cranks had better vibration dampening than the forged steel cranks. The biggest problem was fatigue failure at the ends of the crank pins. That was solved by a rather generous radius between the throw and the crank pin. I know that most small block Chevy and Ford engines were cast iron. As I recall, they mostly used class 65 to 80 of cast ironfor them.
The Enco, and most other easy available, iron is class 40, but I think it would be suitable for most model engines that will not be highly loaded. I have not used it for a crankshaft.